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91.
A resonance enhanced multiphoton ionization (REMPI) mass spectrometer consisting of a tunable laser unit (Nd:YAG pump laser and OPO) and a reflectron mass spectrometer have been upgraded to cope with the difficult conditions such as vibrations, temperature fluctuations and dust, prevailing in an incinerator. On-line measurements of the raw gas have been carried out at the municipal waste incinerator in Stuttgart. Although this test series could not be completed the results are encouraging. They show that wavelength resolution can provide valuable information beyond the one obtainable by fixed frequency REMPI. Examples discussed include separation of interferants to the aniline signal and identification of phenantrene. 相似文献
92.
Cardelino C Chang M St John J Murphey B Cordle J Ballagas R Patterson L Powell K Stogner J Zimmer-Dauphinee S 《Journal of the Air & Waste Management Association (1995)》2001,51(8):1227-1236
Ozone prediction has become an important activity in many U.S. ozone nonattainment areas. In this study, we describe the ozone prediction program in the Atlanta metropolitan area and analyze the performance of this program during the 1999 ozone-forecasting season. From May to September, a team of 10 air quality regulators, meteorologists, and atmospheric scientists made a daily prediction of the next-day maximum 8-hr average ozone concentration. The daily forecast was made aided by two linear regression models, a 3-dimensional air quality model, and the no-skill ozone persistence model. The team's performance is compared with the numerical models using several numerical indicators. Our analysis indicated that (1) the team correctly predicted next-day peak ozone concentrations 84% of the time, (2) the two linear regression models had a better performance than a 3-dimensional air quality model, (3) persistence was a strong predictor of ozone concentrations with a performance of 78%, and (4) about half of the team's wrong predictions could be prevented with improved meteorological predictions. 相似文献
93.
Identifikation der kfz-bürtigen Schadstoffbelastung mit Hilfe der Verh?ltnisse der stabilen Isotope von Kohlenstoff und Schwefel 总被引:1,自引:0,他引:1
Tobias Türcke Stefan Norra Doris Stüben Zsolt Berner und Markus Leosson 《Umweltwissenschaften und Schadstoff-Forschung》1999,11(3):127-133
Zusammenfassung Reifen-, Ru?-, Motoren?l-, Asphalt-, Plastik- und Lackproben aus dem Stra?enverkehr wurden auf ihre Kohlenstoff- und Schwefel-isotopenverh?ltnisse
mit dem Ziel untersucht, die Frage zu beant-worten, ob diese Isotopenverh?ltnisse als Indikatoren für die Belastungssituation
und die Schadstoffquellen bei der Untersuchung von stra?ennahen B?den eingesetzt werden k?nnen. Die δ11C-Werte der technischen Substrate lagen zwischen-30‰ und-18‰ relativ zum PDB-Standard, Dabei zeigte sich aufgrund der unterschiedlichen
Herstellungsverfahren eine deutliche Abgrenzung der Substrate untereinander. Asphalt hatte Werte zwischen-23 und-18‰, Ru?
zwischen -27 und -22‰ Die Ru?proben unterschieden sich je nach Art des verwendeten Kraftstoffs. Plastik, Lack und Motor?le
zeigten ?hnliche δ13C-Werte, die zwischen-30 und-27‰ lagen. Reifen haben relativ konstante δ13C-Werte um -26‰ Der Einflu? des Stra?enverkehrs auf die δ13C-Werte im Stra?ensediment und in stra?ennahen B?den konnte anhand verschiedener Kohlenstoffspezies an einem Transekt an einer
Landstra?e aufgezeigt werden. Ein Vergleich mit verkehrstypischen Schwermetallemissionen ergab bei einzelnen Kohlenstoffspezies
einen ?hnlichen Verlauf der Schwermetallkonzentrationen und der δ13C-Werte.
Die δ34S-Werte lagen zwischen -6 und +8‰ relativ zum CDT-Standard. Eine Abgrenzung der Substrate in ihren δ14S-Werten war hierbei nicht m?glich.
相似文献
94.
A dynamic system based on the water/air equilibrium at the interface within the length of a microporous tube has been used to determine experimentally the Henry's law constants (HLC) of two pesticides: metolachlor and diazinon. The measurements were conducted over the temperature range 283-301 K. At 293 K, HLCs values are (42.6+/-2.8) x 10(3) (in units of M atm(-1)) for metolachlor and (3.0+/-0.3)x10(3) for diazinon. The obtained data were used to derive the following Arrhenius expressions: HLC=(3.0+/-0.4) x 10(-11) exp((10,200+/-1,000)/T) for metolachlor and (7.2+/-0.5) x 10(-15) exp((11,900+/-700)/T) for diazinon. At a cumulus cloud temperature of 283 K, the fractions of metolachlor and diazinon in the atmospheric aqueous phase are about 57% and 11% respectively. In order to evaluate the impact of a cloud on the atmospheric chemistry of both studied pesticides, we compare also their atmospheric lifetimes under clear sky (tau(gas)), and cloudy conditions (tau(multiphase)). The calculated multiphase lifetimes (in units of hours) are significantly lower than those in gas phase at a cumulus temperature of 283 K (in parentheses): metolachlor, 0.4 (2.9); diazinon, 1.9 (5.0). 相似文献
95.
Sylvain Giroud Alina L. Evans Isabelle Chery Fabrice Bertile Georg Tascher Justine Bertrand-Michel Guillemette Gauquelin-Koch Jon M Arnemo Jon E. Swenson Etienne Lefai Stéphane Blanc Chantal Simon 《Die Naturwissenschaften》2018,105(9-10):58
Polyunsaturated fatty acids (PUFAs) exert several important functions across organ systems. During winter, hibernators divert PUFAs from oxidation, retaining them in their tissues and membranes, to ensure proper body functions at low body temperature. PUFAs are also precursors of eicosanoids with pro- and anti-inflammatory properties. This study investigated seasonal changes in eicosanoid metabolism of free-ranging brown bears (Ursus arctos). By using a lipidomic approach, we assessed (1) levels of specific omega-3 and omega-6 fatty acids involved in the eicosanoid cascade and (2) concentrations of eicosanoids in skeletal muscle and blood plasma of winter hibernating and summer active bears. We observed significant seasonal changes in the specific omega-3 and omega-6 precursors. We also found significant seasonal alterations of eicosanoid levels in both tissues. Concentrations of pro-inflammatory eicosanoids, such as thromboxane B2, 5-hydroxyeicosatetraenoic acid (HETE), and 15-HETE and 18-HETE, were significantly lower in muscle and/or plasma of hibernating bears compared to summer-active animals. Further, plasma and muscle levels of 5,6-epoxyeicosatrienoic acid (EET), as well as muscle concentration of 8,9-EET, tended to be lower in bears during winter hibernation vs. summer. We also found lower plasma levels of anti-inflammatory eicosanoids, such as 15dPGJ2 and PGE3, in bears during winter hibernation. Despite of the limited changes in omega-3 and omega-6 precursors, plasma and muscle concentrations of the products of all pathways decreased significantly, or remained unchanged, independent of their pro- or anti-inflammatory properties. These findings suggest that hibernation in bears is associated with a depressed state of the eicosanoid cascade. 相似文献
96.
St. v. Náray-Szabó 《Die Naturwissenschaften》1943,31(16-18):202-203
97.
F. Stöckmann 《Die Naturwissenschaften》1952,39(11):246-254
98.
W. Bader G. Becker M. Kiese Hans Ulrich Wilhelm Simon M. Czerny F. Stöckmann 《Die Naturwissenschaften》1952,39(15):356-360
99.
100.